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Epitaxy of perovskite oxide ferroelectric heterostructures with large lattice misfit is crucial for numerous emerging applications. Here we demonstrate cube-on-cube-type epitaxial growth of BaTiO3 films on strongly mismatched (001)SrTiO3 single-crystal substrates for the films with thicknesses significantly larger than that of misfit relaxation. The films experience strain originating from the film-substrate...
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