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The theory of statistical-mechanical lattice-gas modeling of adsorption is reviewed and shown to be applicable to a range of electrochemical problems dominated by effective, lateral adsorbate-adsorbate interactions. A general strategy for applying the method to specific systems is outlined, which includes microscopic model formulation, calculation of zero-temperature phase diagrams, numerical calculation...
Oxide films have been formed electrochemically at several metallic substrates, including base metals such as a new Al-based microcrystalline alloy (Al-Fe, V, Si) and at polycrystalline Pd electrodes. The Al-based materials were oxidized in sulfuric acid media in order to attempt to form adherent and strong anodic oxide films. The cyclic voltammetry and current transients indicated more active electrochemistry...
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