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One intriguing feature of many porous MOFs is their stimulus‐induced flexibility, which makes them unique compared to standard adsorbents. Here we propose an innovative concept to achieve an efficient kinetic separation of species with similar properties by the mechanical fine‐tuning of the pore architecture of the flexible zeolitic imidazolate framework ZIF‐8. This unprecedented approach was applied...
Finding appropriate stimuli for controlling the breathing behavior of flexible metal–organic frameworks (MOFs) is highly challenging. Herein, we report the solvent‐induced changes in the particle size and stability of different breathing phases of the MIL‐53 series, a group of flexible MOFs. A water/dimethylformamide (DMF) ratio is tuned to synthesize members of the MIL‐53 series which have different...
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