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A number of model Diels‐Alder (D‐A) cycloaddition reactions (H2CCH2 + cyclopentadiene and H2CCHX + 1,3‐butadiene, with X = H, F, CH3, OH, CN, NH2, and NO) were studied by static (transition state ‐ TS and IRC) and dynamics (quasiclassical trajectories) approaches to establish the (a)synchronous character of the concerted mechanism. The use of static criteria, such as the asymmetry of the TS geometry,...
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