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The mechanisms and ionic product distributions related to multiple channels of the X−+CH3ONO2 (X=NCCH2, CH3C(O)CH2, and PhCH2) gas phase reactions were investigated at the B2PLYP/6–311+G(3df,2p)//MP2/6–31+G(d,p) level of theory. The reaction channels are bimolecular nucleophilic displacements at either the carbon (SN2@C) or nitrogen (SN2@N) centers and a proton abstraction followed by dissociation...
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