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NMR study of the organic conductor, (CH 3 ) 4 P[Pd(dmise) 2 ] 2 has been performed. It was found that this compound exhibits a magnetic transition at 30 K. The transition temperature was higher than that of the isostructural sulfur analog, β-(CH 3 ) 4 N[Pd(dmit) 2 ] 2 at ambient pressure (12 K). The electronic states in the insulating...
Physical properties and electronic structures of molecular conductors (cation) [Pd(dmit) 2 ] 2 (cation = Me 4 Z, Et 2 Me 2 Z; Z = N, P, As, and Sb) are described. The Pd(dmit) 2 salts form a unique two-band system. The narrow and two-dimensional HOMO (anti-bonding) band is thought to form the half-filled conduction band. The insulating state under ambient...
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