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2,4,6‐Tridehydropyridinium cation (7) undergoes three consecutive atom or atom group abstractions from reagent molecules in the gas phase. By placing a π‐electron‐donating hydroxyl group between two radical sites, their reactivity can be quenched by enhancing their through‐space coupling via a favorable resonance structure. Indeed, 3‐hydroxy‐2,4,6‐tridehydropyridinium cation (8) abstracts only one...
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