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The tetracationic cyclophane, cyclobis(paraquat‐p‐phenylene), also known as the little blue box, constitutes a modular receptor that has facilitated the discovery of many host–guest complexes and mechanically interlocked molecules during the past 35 years. Its versatility in binding small π‐donors in its tetracationic state, as well as forming trisradical tricationic complexes with viologen radical...
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