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The catalytic (propane dehydrocyclization) and reduction behaviors of near 1:1 cation (Ga, In)/framework‐Al MFI zeolites were examined under conditions where the materials were initially either in fully protonated or zero−protonated states. Reductions at appropriate temperatures proceeded up to ∼100% exchange of protons for reduced univalent cations. Further aqueous exchange of alkali (K+>) or...
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