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Sulfide solid electrolytes (SSEs) for all‐solid‐state Li metal batteries (ASSLMBs) are attracting increasing attention due to their ultrahigh ionic conductivity and good machinability. However, current SSEs generally suffer from inferior Li metal compatibility and poor air‐stability, which severely impede their practical applications for ASSLMBs. Herein, novel argyrodite‐based SSEs of Li6+2xP1−xBi...
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