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Supramolecular polymers based on benzene‐1,3,5‐tricarboxamides (BTAs) functionalized with an L‐ or D‐proline moiety display high catalytic activity towards aldol reactions in water. High turnover frequencies (TOF) of up to 27×10−4 s−1 and excellent stereoselectivities (up to 96 % de, up to 99 % ee) were observed. In addition, the catalyst could be reused and remained active at catalyst loadings and...
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