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1H and 13C NMR studies and quantum chemical calculations show the interaction between 2,11‐dithia‐5,6,8,9‐tetramethyl[32](1,4)cyclophane and nitrosonium cation to result in the formation of π‐ and n‐complexes. According to DFT/B3LYP/6‐31G(2d,p) calculations, formation of nitrosonium complexes is a strongly exothermic process both in gas phase and in SO2. Affinity of single‐charged complexes to NO+...
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