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Ultrathin core–shell V3S4@C nanosheets assembled into hierarchical nanotubes (V3S4@C NS‐HNTs) are synthesized by a self‐template strategy and evaluated as general anodes for alkali‐ion batteries. Structural/physicochemical characterizations and DFT calculations bring insights into the intrinsic relationship between crystal structures and electrochemical mechanisms of the V3S4@C NS‐HNTs electrode....
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