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Polymerization and decomposition of C 60 clusters induced by electron injection from a scanning tunneling microscope (STM) tip have been studied experimentally. The tunneling current dependence of polymerization rate and decomposition rate was found to be both linear, indicating that each reaction is caused by injection of a single electron from the STM tip. We propose a model that an...
The tunneling current injection from a tip of scanning tunneling microscope induces chlorine (Cl) hopping motion on Si(111)-(7x7) and Si(100)-(2x1) surfaces, and polymerization of C 60 clusters in crystalline films of C 60 on Si or highly oriented pyrolytic graphite (HOPG) substrates. In all the cases investigated, the injected carriers spread spatially from the injection...
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