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Laser-ionization of molecules is one of the most important processes in the strong-field and attosecond sciences. One of the key mechanisms governing molecular ionization is enhanced ionization, where for diatomic molecules the ionization probability becomes strongly enhanced at a critical internuclear distance [1, 2]. Experiments on polytatomic molecules have revealed remarkably high charge states...
Recently, selective fragmentation of polyatomic molecules using the carrier-envelope phase (CEP) of few-cycle ionizing laser pulses as the control parameter [1] has been demonstrated [2]. It was shown that the underlying mechanism is selective removal of specific (inner-valence shell) electrons, which puts the molecule into a dedicated dissociative electronic state from which the molecule then fragments...
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