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High interfacial impedance is a major obstacle in the application of solid‐state Li metal batteries (SSLMBs). Understanding the atomic‐scale structure of the interfaces in SSLMBs is thus critical to their practical implementations. However, due to the beam sensitivity of battery materials, such information is not accessible by conventional electron microscopy (EM). Herein, by using cryogenic‐EM (cryo‐EM),...