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To significantly advance the bio‐electrochemical CO2‐conversion rate and unfold the correlation between the abiotic electrode and the attached microorganisms, an atomic‐nanoparticle bridge of Co‐N4@Co‐NP crafted in metal–organic frameworks‐derived nanosheets is integrated with a model methanogen of Methanosarcina barkeri (M. barkeri). The direct bonding of N in Co‐N4 and Fe in member protein of Cytochrome...
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