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The formation of carbonate in neutral/alkaline solutions leads to carbonate crossover, severely reducing carbon dioxide (CO2) single pass conversion efficiency (SPCE). Thus, CO2 electrolysis is a prospective route to achieve high CO2 utilization under acidic environment. Bimetallic Bi‐based catalysts obtained utilizing metal doping strategies exhibit enhanced CO2‐to‐formic acid (HCOOH) selectivity...
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