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With controllable mass transfer and special optical properties, plasmonic nanopores may be applied as a nanodevice and possibly create a new generation of single molecule detection technique based on plasmon‐enhanced spectra. In the present study, gold nanoparticles self‐assemble into a gold porous sphere (GPS) on the tip of a glass nanopipette with the help of i‐motif DNA thiolated by both ends as...
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