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Compounds of GeII are shown for the first time to function as superbases. Two B(N=PiPr3)2 groups attached to a germanium(II) center show a gas‐phase proton affinity of 296.2 kcal mol−1, which is close to the range of a hyperbase as revealed by B3LYP‐D3/6‐31G(2d,p) level of theory. These DFT calculations showed better agreement of geometrical parameters for the reported stable germylene compound 1...
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