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The most successful lithium‐ion batteries (LIBs) based on ethylene carbonate electrolytes and graphite anodes still suffer from severe energy and power loss at temperatures below −20 °C, which is because of high viscosity or even solidification of electrolytes, sluggish de‐solvation of Li+ at the electrode surface, and slow Li+ transportation in solid electrolyte interphase (SEI). Here, a coherent...
In view of their high lithium storage capability, phosphorus‐based anodes are promising for lithium‐ion batteries. However, the low reduction potential (0.74 V versus Li+/Li) of the commonly used ethylene carbonate‐based electrolyte does not allow the early formation of a solid electrolyte interphase (SEI) prior to the initial phosphorus alloying reaction (1.5 V versus Li+/Li). In the absence of a...