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For Bi0.5Na0.5TiO3 (BNT)‐based materials, the effective way of composition modification to solve the drawback of considerable remanent strain (Srem) and achieve high electrostrain appeals intensive research interest, which often accompanies by a high electric field threshold to trigger the transition from ergodic relaxor (ER) state to ferroelectric (FE) state. Here, a unipolar electrostrain of 0.40%...