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Sr2IrO4 exhibits a novel insulating state assisted by spin-orbit interactions. A series of polycrystalline samples of Sr2−xIrO4 have been synthesized. It is found that deep Sr-vacancies of Sr2−xIrO4 greatly reduce the rotation of IrO6 octahedral, and more importantly, a significant structural change occurs around x = 0.48 in both the lattice constants and the Ir−O2 bond length. An insulator-metal...
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