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By virtue of high affinity of Gadolinium(III) with fluoride, a novel MRI/fluorescence bimodal probe was prepared by self-assembly of Gd(III) based contrast agent with the coumarin-based fluorophore (CL). Upon addition of fluoride ion (F−) to the aqueous solution of EDTA-Gd(III)-CL, the replacement of coordination CL occurs, realizing switch-on both the longitudinal relaxivity (r1) and fluorescence...
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