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Piperazine hexahydrate (PI) and diethylenetriamine penta(methylene phosphonic acid) (DTPMP) are used to synthesize flame‐retardant PI‐DTPMP through supramolecular reaction. The incorporation of PI‐DTPMP simultaneously improves the mechanical and flame‐retardant properties of epoxy resin (EP). With only 5 wt% loading of PI‐DTPMP, EP composites show excellent flame retardancy with a limiting oxygen...
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