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In our experimental work on shape-selective isopropylation of naphthalene, the selectivity for 2,6-diisopropylnaphthalene (2,6-DIPN) and the ratio of 2,6-DIPN to 2,7-DIPN were increased by mordenite catalyst dealumination. However, it was not clear whether the differentiation between the two isomers was caused by their differences in molecular dimensions or in electronic properties. In this work we...
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