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An integrated, selective interlayer structure is developed to further mitigate the diffusion of polysulfides, simply by coating the surface of a C–S cathode with a graphene/TiO2 film. It is found that the application of the graphene/TiO2 film as an interlayer enables the porous carbon nanotubes–S cathode to exhibit a high reversible specific capacity and extraordinarily excellent cycling stability...
An integrated, selective graphene/TiO2 interlayer structure is developed by Z. Yang, S. Huang, and co‐workers on page 2891 to further mitigate polysulfide (PS) diffusion. In this rational design, the porous graphene affords an additional electrically conductive network and physically traps PS; as an added bonus, the TiO2 in the graphene/TiO2 barrier film further chemically suppresses the dissolution...
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