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Despite the known efficacy of CeO2 as a promoter in alkaline hydrogen evolution reaction (HER), the underlying mechanism of this effect remains unclear. CoS2, a pyrite‐type alkaline HER electrocatalyst, suffers from sluggish HER kinetics and severe catalyst leaching due to its weak water dissociation kinetics and oxygen‐related corrosion. Herein, it is demonstrated that the interfacial Lewis acid–base...
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