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Designing new forms of ligands and their sandwich‐type analogs is the beginning of building multidecker metallic sandwich clusters and their infinite one‐dimensional molecular wires. Here, we report on two binary B–S clusters: C2v B4S4 (1, 1A1) and D2h B4S4– (2, 2B2u) with rhombic B2S2 as the core are their global minimum structures based upon global searches and electronic structure calculations...
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