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The spin Hamiltonian parameters (g factors, hyperfine structure constants and superhyperfine parameters) and local structures for Ag2+ centers in AgCl and KCl crystals are theoretically studied using the high-order perturbation formulas for a tetragonally elongated 4d9 cluster. The impurity centers undergo relative elongations (≈0.05 Å and 0.23 Å for Ag2+ in AgCl and KCl, respectively) along the C...
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