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The Raman spectrum of PuO2 was measured up to 13,000 cm−1 with three different laser excitation wavelengths spanning the resonance (405 nm), near‐resonance (457 nm), and preresonance (514 nm) energy range. Approximately 26 never‐before‐seen bands were observed between 3500 and 13,000 cm−1. Given the very high energy of the Raman shifts of these bands and the relative insensitivity of their spectral...
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