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Rhenium disulfide (ReS2) holds expansive perspective in photocatalytic water‐splitting field, but its H2‐production rate is severely impeded by the strong hydroxyl (OHad) adsorption on catalytic Re atoms. Herein, an ingenious strategy about charging d‐orbital electrons of ReS2+x cocatalyst by integrating metallic Au is explicitly clarified to effectively accelerate OHad desorption for promoting alkaline...