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The removal of low concentration N2 is of great significance and challenging in the industrial production of high‐purity O2. Herein, a chromium‐based metal–organic framework, namely, TYUT‐96Cr, is reported, which has an unprecedented N2 capture capacity of 37.46 cm3 cm−3 and N2/O2 (5:95, v/v) selectivity up to 26.95 (298 K and 1 bar), thus setting new benchmarks for all reported metal–organic frameworks...
Spatial Structure Reconstruction
In article number 2100866, Jiangfeng Yang, Libo Li, and co‐workers, through optimized spatial structure reconstruction, build TYUT‐96Cr, composed of three kinds of small pore cages using Cr and trimesic acid. Benefitting from the high‐density open Cr sites in the structure, this material features record N2 adsorption volume capacity and N2/O2 separation selectivity,...
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