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Low‐temperature performance of lithium‐ion batteries (LIBs) has always posed a significant challenge, limiting their wide application in cold environments. In this work, the high‐performance LIBs working under ultralow‐temperature conditions, which is achieved by employing the weak‐solvation and low‐viscosity isobutyronitrile as a cosolvent to tame the affinity between solvents and lithium ions, is...
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