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The morphology, pore structure and chemical composition of materials are key to supercapacitor performances. To design reasonable morphology and optimize pore size distribution of materials, we employ a combination of sol-gel method and chemical activation with an aid of freeze drying to prepare a three dimensional hierarchical porous pitch-based aerogel (3DHPPA). The aerogel owns hierarchical porous...
Two-dimensional poly(triazine imide) nanosheets have attracted increasing attention due to the diverse functionalities, however, it remains a challenge to synthesize poly(triazine imide) nanosheets directly from molecular monomers. Here, a novel bottom-up ionothermal method of high efficiency was developed for the synthesis of ultrathin amorphous poly(triazine imide) (aPTI) nanosheets from molecular...
Orientation-induced crystallization is a widely applied method of forming crystal with highly oriented structure. Here, we reported a promising matrix for orientation-induced crystallization–carbon dots (CDs), who exhibited high lattice-matching with Cu crystal. First, CDs induce self-assembly of Cu nanoparticles through organics-inorganics interface interaction, forming self-assembled mesocrystal...
The H2O molecule dissociation on the alkali-earth (Ba and Mg) or transition-metal (Ti)-embedded nitrogen-doped graphene was studied systematically using first-principles calculation. The metal-embedded nitrogen-doped graphene (MN4-graphene) (M = Ba, Mg and Ti) membranes are good candidates for single-atom catalysts (SACs), because the single metal atom can be strongly trapped in the divacancy of the...
We demonstrate a general and facile method to fabricate all-solid-state flexible micro-supercapacitors (MSCs) with micropatterned multi-walled carbon nanotube (MWNT) electrodes via mask-free micro-plasma-jet etching in ambient conditions. Localized pulsed plasma jet etches the MWNTs rapidly and produces the interdigitated electrode patterns by scanning. This mask-free patterning technique is easy...
Carbon dots (CDs) has shown exciting potential in the field of bioscience and biotechnology due to their low toxicity, biological and ecological friendliness and desirable performance characteristics of quantum dots (QDs). However, the effects of CDs on viruses are still largely unknown. In this study, we investigate the effect of CDs on the replication of virus by using pseudorabies virus (PRV) and...
We present joint experimental and theoretical investigations of the deep-ultraviolet Raman scattering spectra of monolayer graphene thin films. We found that upon a 266nm laser excitation, while the G mode remains pronounced, the G′ mode is not observed. The G′ mode exhibits distinctive linewidth broadening towards the ultraviolet frequency region. The peak intensity ratio of the G′ and G modes increases...
Fluorinated graphene, which combines the unique properties of graphite fluoride and graphene, has attracted considerable attention in recent years. Here, we developed a facile, efficient, and scalable method for high-yield exfoliation of graphite fluoride into fluorinated graphene (fluorographene) nanosheets. The exfoliation approach consists of solid ball milling of graphite fluoride with ammonia...
Hierarchically porous carbon materials have many important technological applications; however, most of them were fabricated using either expensive materials or complicated procedures. Based on a general chelate-assisted multi-component co-assembly strategy, nitrogen-doped hierarchically porous carbon materials were fabricated by using Al-based composite and commercial triblock copolymer Pluronic...
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