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A new strategy for the construction of crystalline supermolecular rotors is presented. We obtained the hybrid crystal [(18‐Crown‐6)K]3[NH2(CH3)2]2(Bi2Cl11)·2DMF (1) by introducing the flexible 18‐crown‐6 into the inorganic [Bi2Cl11]5– binuclear anion cluster lattice through the KCl (screw) to connect the organic molecule with inorganic component, in which the coordinated DMF (N,N‐Dimethylformamide)...