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Bithiophene imide (BTI)‐based polymers have been promising photovoltaic materials due to their high mobility and tunable energy levels. However, BTI polymers have rarely been revisited since organic solar cells (OSCs) entered the era of non‐fullerene electron acceptors (NFEA) likely owing to their incompatibility with NFEAs. Herein, fine‐tuning the aggregation and orientation of BTI‐based donor‐π‐acceptor...
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