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Transition‐metal catalyzed C—C bond activation is a formidable challenge owing to the high bond energy. We report here a novel palladium‐catalyzed C—C bond activation manner of methylenecyclobutanes followed by subsequent Suzuki cross‐coupling reaction affording multisubstituted indanes. The tandem reaction process involves intramolecular carbopalladation of double bond, β‐carbon elimination and intermolecular...
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