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A rhodium/photoredox dual catalyzed regiodivergent α‐allylation of amines is described. As an atom‐economic and efficient method, alkynes and allenes are used as allylic electrophile surrogates in this novel protocol. With different reaction conditions, synthetically useful branched or linear homoallylic amines could be synthesized in good to excellent yields and regioselectivity. This straightforward...
Eine Reihe von Übergangsmetall‐Katalysatoren ist in der Lage, terminale und interne Alkine intermediär in entsprechende Allylmetall‐Verbindungen zu überführen, die ihrerseits elektrophile oder nukleophile Reaktivitäten aufweisen können. Während klassische Methoden zur Herstellung von Allylmetall‐Spezies oftmals von der Bildung stöchiometrischer Mengen an Nebenprodukten begleitet sind, ermöglicht der...
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