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Light‐guided soft actuators with dynamic polymer networks have drawn much attention in recent years. However, the application of such actuators is limited by their synthetic strategies, polymer structures, and shape‐morphing modes. This work reports a new class of liquid crystalline elastomer (LCE) actuators crosslinked by mussel‐inspired catechol‐Fe (III) complexes. The actuators are mechanically...
Shape memory polymers (SMPs) with the permanent shape reconfiguration capability have received much research interest because they are capable of diversified tasks and the ability to work in conditions that required complex geometry. However, most of such SMPs are thermally triggered, which limits their applications. Inspired by reversible mussel adhesive protein chemistry, NIR light‐triggered SMPs...
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