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The stable and efficient integration of molecular catalysts into p‐type semiconductor materials is a contemporary challenge in photoelectrochemical fuel synthesis. Here, we report the combination of a phosphonated molecular Ni catalyst with a TiO2‐coated La5Ti2Cu0.9Ag0.1S5O7 photocathode for visible light driven H2 production. This hybrid assembly provides a positive onset potential, large photocurrents,...
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