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Li‐rich Mn‐based layered oxides (LRLOs) with ultrahigh specific capacities are promising cathode materials for high energy density lithium‐ion batteries. Nevertheless, severe irreversible oxygen release, structure degradation, capacity and voltage attenuation hinder their commercialization due to the uncontrollable oxygen redox chemistry originated from unhybridized O 2p orbitals. Herein, a strategy...
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