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A unique feature of multifunctional asymmetric catalysts is described. Catalytic asymmetric Michael reaction of cyclic enones with Horner-Wadsworth-Emmons reagents proceeds efficiently by use of an aluminum-lithium-BINOL complex that is activated by an addition of alkali metal reagent. In addition, rare earth-3-hydroxymethyl-BINOL complexes promote asymmetric epoxidation of cis-enones to afford cis-epoxyketones...
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