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The elusive, multiple fully extended (2.05‐helix) peptide conformation was searched with a series of Cα,α‐diethylglycine homo‐oligomers (n = 1 to 5) functionalized by an electron transfer (ET) donor···acceptor (D···A) pair in acetonitrile and chloroform solutions. In the former solvent, all peptides investigated were shown to populate the 310‐helix conformation, whereas in chloroform the two shortest...
The photocurrent generation process of peptide‐based self‐assembled monolayers immobilized on a gold electrode can be enhanced by functionalizing the peptide scaffold with UV‐Vis absorbing groups (antenna effect). Moreover, the coupling between the photoactive layer and the conductive substrate can be controlled by changing the nature of the .peptide/gold interface (junction effect).
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