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The carbon‐to‐silicon switch in formation of bioactive sila‐heterocycles with a silicon‐stereogenic center has garnered significant interest in drug discovery. However, metal‐catalyzed synthesis of such scaffolds is still in its infancy. Herein, a rhodium‐catalyzed enantioselective formal [4+1] cyclization of benzyl alcohols and benzaldimines has been realized by enantioselective difunctionalization...
The carbon‐to‐silicon switch in formation of bioactive sila‐heterocycles with a silicon‐stereogenic center has garnered significant interest in drug discovery. However, metal‐catalyzed synthesis of such scaffolds is still in its infancy. Herein, a rhodium‐catalyzed enantioselective formal [4+1] cyclization of benzyl alcohols and benzaldimines has been realized by enantioselective difunctionalization...
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