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The daphnezomine A‐type subfamily of Daphniphyllum alkaloids structurally features a unique aza‐adamantane core skeleton and anticipates efficient strategies for completing their syntheses to thoroughly investigate their biological activities. Herein, divergent total syntheses of (−)‐daphnezomines A and B and (+)‐dapholdhamine B have been accomplished in 16–20 steps from a known epoxide via rapid...
The daphnezomine A‐type subfamily of Daphniphyllum alkaloids structurally features a unique aza‐adamantane core skeleton and anticipates efficient strategies for completing their syntheses to thoroughly investigate their biological activities. Herein, divergent total syntheses of (−)‐daphnezomines A and B and (+)‐dapholdhamine B have been accomplished in 16–20 steps from a known epoxide via rapid...
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