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Die dative Bindung …… zwischen dem hochreaktiven Silylkation und Wasser in protoniertem Silanol wurde von O. Dopfer und Mitarbeitern in ihrer Zuschrift auf S. 2969 mithilfe von Infrarotspektroskopie und Dichtefunktionalrechnungen untersucht. Die Ergebnisse bezüglich Struktur und Bindungsverhältnissen und die Infrarotsignatur dieses einfachsten Silanol‐Kations könnten seine Identifizierung erleichtern,...
We report the spectroscopic characterization of protonated monosilanol (SiH3OH2+) isolated in the gas phase, thus providing the first experimental determination of the structure and bonding of a member of the elusive silanol family. The SiH3OH2+ ion is generated in a silane/water plasma expansion, and its structure is derived from the IR photodissociation (IRPD) spectrum of its Ar cluster measured...
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