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The α‐CsPbI3 nanocrystals (NCs) easily transform into yellow non‐perovskite, accompanying with declining photoelectric properties that restricting their practical applications in diverse fields. Herein, the highly luminescent and robust α‐CsPbI3 NCs is achieved through engineering the lattice symmetry of perovskite, enabled by the synergistic effect of NO3− ion passivation and Ca2+ ion doping. The...
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