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Supported ionic liquid phase (SILP) catalysis enables a highly efficient, Ru‐based, homogeneously catalyzed water‐gas shift reaction (WGSR) between 100 °C and 150 °C. The active Ru‐complexes have been found to exist in imidazolium chloride melts under operating conditions in a dynamic equilibrium, which is dominated by the [Ru(CO)3Cl3]− complex. Herein we present state‐of‐the‐art theoretical calculations...
H2‐Gas kann bei niedrigen Temperaturen durch eine rutheniumkatalysierte Wassergas‐Shift‐Reaktion (WGSR) freigesetzt werden. Basierend auf einem kombinierten theoretischen und experimentellen Ansatz präsentieren D. M. Smith und Mitarbeiter in ihrer Zuschrift auf S. 751 einen neuen WGSR‐Mechanismus mit chloridreichen anionischen Rutheniumcarbonylkomplexen. Die Ergebnisse stützen sich auf kinetische...
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