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A highly enantioselective Pd‐catalyzed amination of allenyl phosphates generating 2,3‐allenyl amines with central chirality has been developed. Under the optimized conditions, chiral 2,3‐allenyl amines with or without (an) additional CC double or triple bond(s) have been prepared at 0 °C with up to 90 % yield and 94 % ee by identifying (R)‐3,4,5‐(MeO)3‐MeOBIPHEP as the ligand.
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